Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake

LIU En-feng; SHEN Ji; ZHU Yu-xin; XIA Wei-lan; PAN Hong-xi; JIN Zhang-dong

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Article Navigation > Acta Sedimentologica Sinica > 2004 > 22(3): 507-512

LIU En-feng, SHEN Ji, ZHU Yu-xin, XIA Wei-lan, PAN Hong-xi, JIN Zhang-dong. Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake[J]. Acta Sedimentologica Sinica, 2004, 22(3): 507-512.

Citation:

LIU En-feng, SHEN Ji, ZHU Yu-xin, XIA Wei-lan, PAN Hong-xi, JIN Zhang-dong. Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake[J]. Acta Sedimentologica Sinica, 2004, 22(3): 507-512.

Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake

1.
Nanjing Institute of Geography & Limnology,Chinese Academy of Sciences,Nanjing 210008;
2.
Graduate School of the Chinese Academy of Sciences,Beijing 100039

Received Date: 2003-06-16
Rev Recd Date: 2004-09-01
Publish Date: 2004-09-10

Abstract

Sedimentation rates,element concentrations and grain sizes distribution of Cores MS and DLS sediments from Taihu Lake are investigated.According to ¹³⁷ Cs dating,modern accumulation rates of Cores MS and DLS are 1.7 mm/a and 0.9mm/a.The pollution history of Taihu Lake is studied based on the geochemical characteristics in Core MS sediments.Pb,Zn,As,Hg,Mn and Ni are the main pollution heavy metals,which have different pollution history and pollution degree.The concentration of As in sediments increased since 1930s'due to the private industries development,and that of Hg increased since 1940s',which is the important pollution element due to the bio-accumulative effect.Pb,Zn,Ni and Mn pollution began at late 1970s'and the concentration in sediments became higher as As and Hg.The concentration of TP increased since 1940s',and that of TN and TOC was from late 1970s',which have close correlation with the eutrophication of lake.The history of elements pollution is correspondent with the economy development in the catchment of Taihu Lake.
- Taihu Lake,
- heavy metals,
- total nitrogen,
- total phosphorus,
- total organic carbon,
- pollution history

References

[1]	Von Gunten H R,Sturm M,Moser R N.200-year record of metals in lake sediments and nature background concentrations.Environmental Science and Technology,1997,31:2193～2197
[2]	张学恕.中国长江下游经济发展史.南京:东南大学出版社,1990.271～301,683～737 [Zhang Xueshu.History of economic development in the lower reaches of the Yangtse River.Nanjing: Southeast University Press,1990.271～301,683～737]
[3]	谢红彬,陈雯.太湖流域制造业结构变化对水环境演变影响分析-以苏锡常地区为例.湖泊科学,2002,14(1):53～39 [Xie Hongbin, Chen Wen.Impacts of change of industrial structure on the water environment in Taihu Basin:A case study of Suzhou-Wuzi-Changzhou district.Journal of Lake Sciences,2002,14(1):53～39]
[4]	戴秀丽,孙成.太湖沉积物中重金属污染状况及分布特征探讨.上海环境科学,2001,20(2):71～74 [Dai Xiuli, Sun Cheng.The characteristics of heavy metals distribution and pollution in sediment from Lake Taihu.Shanghai Environmental Sciences, 2001,20(2):71～74]
[5]	王海,王春霞,王子健.太湖表层沉积物中重金属的形态分析.环境化学,2002,21(5):430～435 [Wang Hai,Wang Chunxia,Wang Zijian.Speciations of heavy metals in surface sediment of Taihu Lake.Environmental Chemistry,2002,21(5):430～435]
[6]	袁旭音,陈骏,季峻峰,等.太湖沉积物和湖岸土壤的污染元素特征及环境变化效应.沉积学报,2002,20(3):427～434 [Yuan Xuyin,Chen Jun,Ji Junfeng,et al.Characteristics and environmental changes of pollution elements in Taihu sediments and soils near the lake.Acta Sedimentologica Sinica,2002,20(3):427～434]
[7]	Li X D,Wai O W H,Li Y S,et al.Heavy metal distribution in sediment profiles of the Pearl River Estuary.Applied Geochemistry,2000,15:567～581
[8]	Lacey E M,King J W,Quinn J G,et al.Sediment quality in Burlington Harbor,Lake Champlain,U.S.A.Water Air & Soil Pollution,2001,126:97～120
[9]	刘英俊,曹励明,李兆麟,等.元素地球化学.北京:科学出版社,1984. 16～19;62～64 [Liu Yingjun,Cao Liming,Li Zhaolin,et al. Element geochemistry.Beijing:Science Press,1984. 16～19;62～64]
[10]	孙顺才,黄漪平.太湖.北京:海洋出版社,1993.5～224 [Sun Shuncai,Huang Yiping.Taihu Lake.Beijng:China Ocean Press,1993.5～224]
[11]	马嘉蕊,邵秘华.锦州湾沉积物芯样中重金属污染及变化动态.中国环境科学,1994,14(1): 22～29 [Ma Jiarui,Shao Mihua.Variation in heavy metal pollution of offshore sedimentary cores in Jinzhou Bay.China Environmental Science,1994,14(1): 22～29]
[12]	郭瑞霞,杨建丽,刘东燕,等.煤热解过程中无机有害元素的变迁规律.环境化学,2002,23(5):100～104 [Guo Ruixia, Yang Jianli, Liu Dongyan, et al.Transformation of Na,K,Pb and Mn during pyrolysis of coal.Environmental Science,2002,23(5):100～104]
[13]	Moon J W,Moon H S,Woo N C,et al.Evaluation of heavy metal contamination and implication of multiple sources from Hunchun basin,northeastern China.Environmental Geology,1999,39(9): 1039～1052
[14]	朱广伟,陈英旭,周根娣.运河(杭州段)沉积物中重金属分布特征及变化.中国环境科学,2001,21(1):65～69 [Zhu Guangwei,Chen Yingxu,Zhou Gengdi.Distribution of heavy metals in the sediments from the Grand Canal(Hangzhou section).China Environmental Science,2001,21(1):65～69]
[15]	冯新斌,洪冰,倪建宇,等.煤中部分潜在毒害微量元素在表生条件下的化学活动性.环境科学学报1999,19(4):433～437 [Feng Xinbin,Hong Bing,Ni Jianyu,et al.Chemical mobility of potentially toxic elements in coal at surface conditions. Acta Scientiae Circumstantiae,1999,19(4):433～437]
[16]	刘桂建,杨萍玥,彭子成,等.兖州矿区煤中某些微量元素的赋存状态研究.地球化学,2002,31(1):85～90 [Liu Guijian,Yang Pingyue,Peng Zicheng,et al. Occurrence of trace elements in coal of Yanzhou Mining District.Geochemica,2002,31(1):85～90]
[17]	李任伟,李禾,李原,等.黄河三角洲沉积物重金属、氮和磷污染研究.沉积学报,2001,19(4):622～629 [Li Renwei,Li He,Li Yuan,et al.Study of the heavy metals,nitrogen and phosphorus contaminants in the sediments of the yellow river delta.Acta Sedimentologica Sinica,2001,19(4):622～629]
[18]	Karin Brack,Rodney L Stevens.Historical pollution trends in a disturbed,estuarine sedimentary, environment,SW Sweden.Environmental Geology,2001,40:1017～1029
[19]	Shen Ji,Ryo Matsumoto,Wang S M.A 3600 years paleoclimatic change inferred from organic ¹³C and TOC/TN of the Gucheng Lake sediments,Southeast China.China J Oceanol Limnol,1997,15(3):279～284
[20]	伍献文.五里湖1951年湖泊学调查.水生生物学集刊,1962,1:63～113 [Wu Wenxian.Limnology investigation of Wuli Lake in 1951.Hydrobiology Quarterly,1962,1:63～113]
[21]	张路,范成新,秦伯强,等.模拟扰动条件下太湖表层沉积物磷行为的研究.湖泊科学,2001,11(1):35～42 [Zhang Lu,Fan Chengxin,Qing Boqiang,et al. Phosphorus release and absorption of surface sediments in Taihu Lake under simulative disturbing conditions.Journal of Lake Science,2001,11(1):35～42]
[22]	隋少峰,罗启芳.武汉东湖底泥释磷特点.环境科学,2001,22(1):102～105 [Sui Shaofeng,Luo Qifang.Release characters of phosphorus from the sediments of East Lake,Wuhan.Environmental Science,2001,22(1):102～105]
[23]	杨清心.太湖水华成因及控制途径初探.湖泊科学,1996,8(1):67～74 [Yang Qingxin.Algal bloom in Taihu Lake and its control. Journal of Lake Sciences,1996,8(1):67～74]
[24]	王万茂,李玉英,朱德明.太湖水土资源保护和经济发展研究.资源开发与市场,1996,12(6):262～264 [Wang Wanmao,Li Yuying,Zhu Deming.Water and soil resources protection with economy development.Resource Development & Market,1996,12(6):262～264]
[25]	William Y B Chang.中国太湖1950年以来主要环境的变化与迅速富营养化的开始.古生物学报,1996,35(2):155～174 [William Y B Chang.Major environmental changes since 1950 and the onset of accelerated eutrophication in Taihu Lake,China.Acta Palaeontologica Sinica,1996,35(2):155～174]
[26]	吴瑞金.湖泊沉积物的磁化率、频率磁化率及其古气候意义.湖泊科学,1993,6(2):128～135 [Wu Ruijin.Magnetic susceptibility and frequency dependent susceptibility of lake sediments and their paleoclimatic implication.Journal of Lake Sciences,1993,6(2):128～135]
[27]	张卫国,俞立中,Hutchison S M.长江口南岸边滩沉积物重金属污染记录的磁诊断方法.海洋与湖沼,2000,31(6):616～623 [Zhang Weiguo,Yu Lizhong.Hutchison S M.Magnetic diagnosis of heavy metal pollution record in coastal sediments on the southern bank of the Yangtze River estuary.Oceanologia et Limnologiasinica,2000,31(6):616～623]

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通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

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Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake

1. Nanjing Institute of Geography & Limnology,Chinese Academy of Sciences,Nanjing 210008;

2. Graduate School of the Chinese Academy of Sciences,Beijing 100039

Received Date: 2003-06-16

Rev Recd Date: 2004-09-01

Publish Date: 2004-09-10

Key words:

Abstract: Sedimentation rates,element concentrations and grain sizes distribution of Cores MS and DLS sediments from Taihu Lake are investigated.According to ¹³⁷ Cs dating,modern accumulation rates of Cores MS and DLS are 1.7 mm/a and 0.9mm/a.The pollution history of Taihu Lake is studied based on the geochemical characteristics in Core MS sediments.Pb,Zn,As,Hg,Mn and Ni are the main pollution heavy metals,which have different pollution history and pollution degree.The concentration of As in sediments increased since 1930s'due to the private industries development,and that of Hg increased since 1940s',which is the important pollution element due to the bio-accumulative effect.Pb,Zn,Ni and Mn pollution began at late 1970s'and the concentration in sediments became higher as As and Hg.The concentration of TP increased since 1940s',and that of TN and TOC was from late 1970s',which have close correlation with the eutrophication of lake.The history of elements pollution is correspondent with the economy development in the catchment of Taihu Lake.

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Reference (27)

[1]	Von Gunten H R,Sturm M,Moser R N.200-year record of metals in lake sediments and nature background concentrations.Environmental Science and Technology,1997,31:2193～2197
[2]	张学恕.中国长江下游经济发展史.南京:东南大学出版社,1990.271～301,683～737 [Zhang Xueshu.History of economic development in the lower reaches of the Yangtse River.Nanjing: Southeast University Press,1990.271～301,683～737]
[3]	谢红彬,陈雯.太湖流域制造业结构变化对水环境演变影响分析-以苏锡常地区为例.湖泊科学,2002,14(1):53～39 [Xie Hongbin, Chen Wen.Impacts of change of industrial structure on the water environment in Taihu Basin:A case study of Suzhou-Wuzi-Changzhou district.Journal of Lake Sciences,2002,14(1):53～39]
[4]	戴秀丽,孙成.太湖沉积物中重金属污染状况及分布特征探讨.上海环境科学,2001,20(2):71～74 [Dai Xiuli, Sun Cheng.The characteristics of heavy metals distribution and pollution in sediment from Lake Taihu.Shanghai Environmental Sciences, 2001,20(2):71～74]
[5]	王海,王春霞,王子健.太湖表层沉积物中重金属的形态分析.环境化学,2002,21(5):430～435 [Wang Hai,Wang Chunxia,Wang Zijian.Speciations of heavy metals in surface sediment of Taihu Lake.Environmental Chemistry,2002,21(5):430～435]
[6]	袁旭音,陈骏,季峻峰,等.太湖沉积物和湖岸土壤的污染元素特征及环境变化效应.沉积学报,2002,20(3):427～434 [Yuan Xuyin,Chen Jun,Ji Junfeng,et al.Characteristics and environmental changes of pollution elements in Taihu sediments and soils near the lake.Acta Sedimentologica Sinica,2002,20(3):427～434]
[7]	Li X D,Wai O W H,Li Y S,et al.Heavy metal distribution in sediment profiles of the Pearl River Estuary.Applied Geochemistry,2000,15:567～581
[8]	Lacey E M,King J W,Quinn J G,et al.Sediment quality in Burlington Harbor,Lake Champlain,U.S.A.Water Air & Soil Pollution,2001,126:97～120
[9]	刘英俊,曹励明,李兆麟,等.元素地球化学.北京:科学出版社,1984. 16～19;62～64 [Liu Yingjun,Cao Liming,Li Zhaolin,et al. Element geochemistry.Beijing:Science Press,1984. 16～19;62～64]
[10]	孙顺才,黄漪平.太湖.北京:海洋出版社,1993.5～224 [Sun Shuncai,Huang Yiping.Taihu Lake.Beijng:China Ocean Press,1993.5～224]
[11]	马嘉蕊,邵秘华.锦州湾沉积物芯样中重金属污染及变化动态.中国环境科学,1994,14(1): 22～29 [Ma Jiarui,Shao Mihua.Variation in heavy metal pollution of offshore sedimentary cores in Jinzhou Bay.China Environmental Science,1994,14(1): 22～29]
[12]	郭瑞霞,杨建丽,刘东燕,等.煤热解过程中无机有害元素的变迁规律.环境化学,2002,23(5):100～104 [Guo Ruixia, Yang Jianli, Liu Dongyan, et al.Transformation of Na,K,Pb and Mn during pyrolysis of coal.Environmental Science,2002,23(5):100～104]
[13]	Moon J W,Moon H S,Woo N C,et al.Evaluation of heavy metal contamination and implication of multiple sources from Hunchun basin,northeastern China.Environmental Geology,1999,39(9): 1039～1052
[14]	朱广伟,陈英旭,周根娣.运河(杭州段)沉积物中重金属分布特征及变化.中国环境科学,2001,21(1):65～69 [Zhu Guangwei,Chen Yingxu,Zhou Gengdi.Distribution of heavy metals in the sediments from the Grand Canal(Hangzhou section).China Environmental Science,2001,21(1):65～69]
[15]	冯新斌,洪冰,倪建宇,等.煤中部分潜在毒害微量元素在表生条件下的化学活动性.环境科学学报1999,19(4):433～437 [Feng Xinbin,Hong Bing,Ni Jianyu,et al.Chemical mobility of potentially toxic elements in coal at surface conditions. Acta Scientiae Circumstantiae,1999,19(4):433～437]
[16]	刘桂建,杨萍玥,彭子成,等.兖州矿区煤中某些微量元素的赋存状态研究.地球化学,2002,31(1):85～90 [Liu Guijian,Yang Pingyue,Peng Zicheng,et al. Occurrence of trace elements in coal of Yanzhou Mining District.Geochemica,2002,31(1):85～90]
[17]	李任伟,李禾,李原,等.黄河三角洲沉积物重金属、氮和磷污染研究.沉积学报,2001,19(4):622～629 [Li Renwei,Li He,Li Yuan,et al.Study of the heavy metals,nitrogen and phosphorus contaminants in the sediments of the yellow river delta.Acta Sedimentologica Sinica,2001,19(4):622～629]
[18]	Karin Brack,Rodney L Stevens.Historical pollution trends in a disturbed,estuarine sedimentary, environment,SW Sweden.Environmental Geology,2001,40:1017～1029
[19]	Shen Ji,Ryo Matsumoto,Wang S M.A 3600 years paleoclimatic change inferred from organic ¹³C and TOC/TN of the Gucheng Lake sediments,Southeast China.China J Oceanol Limnol,1997,15(3):279～284
[20]	伍献文.五里湖1951年湖泊学调查.水生生物学集刊,1962,1:63～113 [Wu Wenxian.Limnology investigation of Wuli Lake in 1951.Hydrobiology Quarterly,1962,1:63～113]
[21]	张路,范成新,秦伯强,等.模拟扰动条件下太湖表层沉积物磷行为的研究.湖泊科学,2001,11(1):35～42 [Zhang Lu,Fan Chengxin,Qing Boqiang,et al. Phosphorus release and absorption of surface sediments in Taihu Lake under simulative disturbing conditions.Journal of Lake Science,2001,11(1):35～42]
[22]	隋少峰,罗启芳.武汉东湖底泥释磷特点.环境科学,2001,22(1):102～105 [Sui Shaofeng,Luo Qifang.Release characters of phosphorus from the sediments of East Lake,Wuhan.Environmental Science,2001,22(1):102～105]
[23]	杨清心.太湖水华成因及控制途径初探.湖泊科学,1996,8(1):67～74 [Yang Qingxin.Algal bloom in Taihu Lake and its control. Journal of Lake Sciences,1996,8(1):67～74]
[24]	王万茂,李玉英,朱德明.太湖水土资源保护和经济发展研究.资源开发与市场,1996,12(6):262～264 [Wang Wanmao,Li Yuying,Zhu Deming.Water and soil resources protection with economy development.Resource Development & Market,1996,12(6):262～264]
[25]	William Y B Chang.中国太湖1950年以来主要环境的变化与迅速富营养化的开始.古生物学报,1996,35(2):155～174 [William Y B Chang.Major environmental changes since 1950 and the onset of accelerated eutrophication in Taihu Lake,China.Acta Palaeontologica Sinica,1996,35(2):155～174]
[26]	吴瑞金.湖泊沉积物的磁化率、频率磁化率及其古气候意义.湖泊科学,1993,6(2):128～135 [Wu Ruijin.Magnetic susceptibility and frequency dependent susceptibility of lake sediments and their paleoclimatic implication.Journal of Lake Sciences,1993,6(2):128～135]
[27]	张卫国,俞立中,Hutchison S M.长江口南岸边滩沉积物重金属污染记录的磁诊断方法.海洋与湖沼,2000,31(6):616～623 [Zhang Weiguo,Yu Lizhong.Hutchison S M.Magnetic diagnosis of heavy metal pollution record in coastal sediments on the southern bank of the Yangtze River estuary.Oceanologia et Limnologiasinica,2000,31(6):616～623]

Heavy Metals and Nutrients Pollution in Sediments of Taihu Lake

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通讯作者: 陈斌, bchen63@163.com

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