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济阳拗陷特殊生物降解油的初步研究

卢鸿 彭平安 徐兴友 张林晔

卢鸿, 彭平安, 徐兴友, 张林晔. 济阳拗陷特殊生物降解油的初步研究[J]. 沉积学报, 2004, 22(4): 694-699.
引用本文: 卢鸿, 彭平安, 徐兴友, 张林晔. 济阳拗陷特殊生物降解油的初步研究[J]. 沉积学报, 2004, 22(4): 694-699.
LU Hong, PENG Ping an, XU Xing you, ZHANG Lin ye. Preliminary Study on the Severely Biodegraded Crude Oil in Jiyang Depression, China[J]. Acta Sedimentologica Sinica, 2004, 22(4): 694-699.
Citation: LU Hong, PENG Ping an, XU Xing you, ZHANG Lin ye. Preliminary Study on the Severely Biodegraded Crude Oil in Jiyang Depression, China[J]. Acta Sedimentologica Sinica, 2004, 22(4): 694-699.

济阳拗陷特殊生物降解油的初步研究

基金项目: 中国科学院创新知识工程项目(KZCX1-SW-18);国家基础研究“973”项目(G1999043308)资助.
详细信息
    作者简介:

    卢鸿 男 1971年出生 副研究员 石油地球化学和有机地球化学

  • 中图分类号: P593

Preliminary Study on the Severely Biodegraded Crude Oil in Jiyang Depression, China

  • 摘要: 济阳拗陷草古100平19井奥陶系储层原油,饱和烃馏分均已损失殆尽,仅残余藿烷系列化合物;同时,芳烃馏分化合物也已损失殆尽,仅残余三芳甾烷系列化合物。上述芳烃化合物俱已损失殆尽的蚀变特征,在相关文献中的报道较为少见。原油中不受水洗作用影响的正构烷烃和不受生物降解作用影响的有机硫化合物(苯并噻吩和二苯并噻吩)均已损失殆尽,显然暗示了原油蚀变是遭受水洗作用和生物降解作用共同作用的结果。原油芳烃馏分的“UCM”鼓包幅度明显大于饱和烃馏分的“UCM”鼓包,暗示了芳烃化合物的降解速率平行甚至超过饱和烃的降解速率。原油中低分子量芳烃化合物的快速降解,暗示了油藏可能是在氧化条件下而非在还原条件下发生蚀变的。
  • [1] Bastin E. Microorganisms in oilfields. Sciences, 1926,63:21~24
    [2] Milner C W D, Rogers M A, Evans C R. Petroleum transformations in reservoirs. Journal of Geochemical Exploration, 1977, 7: 101~153
    [3] Schink B. Degradation of unsaturated hydrocarbons in crude oil by methanogenic enrichment cultures. FEMS Microbiology Ecology, 1985, 31: 69~77
    [4] Aeckersberg F, Bak F, Widdel F. Anaerobic oxidation of saturated hydrocarbons to CO2 by a new type of sulfate-reducing bacterium. Archives of Microbiology, 1991, 156: 5~14
    [5] Wilhelms A, Larter S R, Head I, Farrimond P, et al. Biodegradation of oil in uplifted basins prevented by deep-burial sterilization. Nature, 2001, 411: 1034~1037
    [6] Jobson A, Cook F D, Westlake D W S. Microbial utilization of crude oil. Applied Microbiology and Biotechnology, 1972, 23: 1082~1089
    [7] Stahl W J. Compositional changes and 13C/12C fractionation during the degradation of hydrocarbons by bacteria. Geochimica et Cosmochimica Acta, 1980, 44:1903~1907
    [8] Connan J, Le Thahn K, van der Weide. Alteration of petroleum in reservoirs. Proc. 9th world Pet. Cong., 1975.171~178
    [9] Deroo G., Powell T G, Tissot B, McCrossan R G. The origin and migration of petroleum in the Western Canadian sedimentary basin, Alberta. Geological Survey of Canada Bulletin, 1977, 262: 136
    [10] Rubinstein I, Strausz O P, Spyckerelle C, et al. The origin of the oil sand bitumens of Alberta: a chemical and a microbiological simulation study. Geochimica et Cosmochimica Acta, 1977, 41: 1341~1353
    [11] Jones D M, Douglas G, Wehrung P, et al. The recognition of biodegraded petroleum-derived aromatic hydrocarbons in recent marine sediments. Marine Pollution Bulletin, 1983,14:103~108
    [12] Volkman J K. Biodegradation of aromatic hydrocarbons in crude oils from the Barrow Sub-basin of Western Australia. Organic Geochemistry, 1984, 6: 619~632
    [13] Fisher S J, Alexander R, Kagi R I. Biodegradation of alkylnaphthalenes in sediment adjacent to an offshore petroleum production platform. Polycyclic Aromatic Compounds, 1996, 11:35~42
    [14] Fisher S J, Alexander R, Kagi R I, Oliver G A. Aromatic hydrocarbons as indicators of petroleum biodegradation in North Western Australian reservoirs. In: Purcell P G, Purcell B R, eds. The sedimentary basins of Western Australia 2, Proceedings of Petroleum Exploration Society Symposium. Perth, 1998. 185~194
    [15] Ahmed M, Smith J W, George S C. Effects of biodegradation on Austrlian Permian coals. Organic Geochemistry, 1999, 30(10): 1311~1322
    [16] Van Aarssen B G K, Bastow T P, Alexander R, Kagi RI. Distributions of methylated naphthalenes in crude oils: indicators of maturity, biodegradation and mixing. Organic Geochemistry, 1999.30:1213~1227
    [17] Connan J. Biodegradation of crude oils in reservoirs. In: Brooks J, Welte D, eds. Advances in Petroleum Geochemistry. Vol.1. London:Academic Press, 1984. 299
    [18] 蒋助生. 克拉玛依原油中的降解甾烷和萜烷. 见:有机地球化学和陆相生油. 北京: 石油工业出版社, 1986. 72~82[Jiang Zhusheng, Biodegraded steranes and terpanes in crude oils from Kelamayi Oilfield, NW China. Organic Geochemistry and terrestrial hydrocarbon generation. Beijing: Petroleum Industry Press,1986.72~82]
    [19] 张大江. 克拉玛依原油的生物降解. 石油勘探与开发,1987, 14(4):34~40.[Zhang Dajiang et al. Biodegradation in crude oils from Kelamayi Oildield, NW China. Petroleum exploration and development.1987,14(4):34~40]
    [20] 王屿涛. 准噶尔盆地西北缘稠油生物降解特征. 沉积学报,1994, 12(1):81~87[Wang Yutao. Characteristics of biodegraded heavy oils in northwestern part of Jungar Basin, NW China. Acta Sedimentologica Sinica,1994,12(1):81~87]
    [21] 熊永强, 耿安松, 刘得光. 克拉玛依油田稠油中萜类化合物单体碳同位素组成. 科学通报, 1998, 12:1312~1315[Xiong Yongqiang, Geng Ansong and Liu Deguang. Stable carbon isotopic compositions of compound specific terpanoils for heavy oils in Kelamayi oilfield, NW China. Chinese Bulletin of Sciences. 1998,43(12):1312~1315]
    [22] 宋一涛, 等. 孤东油田生物降解原油的特征及油源勘探. 陆相石油地质文集. 北京: 石油工业出版社,1995[Song Yitao,et al. Characteristics and exploration target of biodegraded oils in Gudong Oilfield, Jiyang Depression. Corpus for terrestrial Petroleum Geology. Beijing: Petroleum Industry Press,1995]
    [23] 熊永强, 耿安松. 辽河油田生物降解原油沥青质热解产物中单体化合物碳同位素组成.地球化学,1998, 6:532~536[Xiong Yongqiang and Geng Ansong. Stable carbon isotopic compositions of compound specific hydrocarbons in perolysed products of asphaltene fraction for biodegraded oils in Liaohe Oilfield. Geochemistry,1998,27(6):532~536]
    [24] 梁春秀, 刘宝柱, 孙万军. 松辽盆地南部的西部斜坡重油特征与油源探讨. 石油勘探与开发, 2002, 2:45~48[Liang Chunxiu, Liu Baozhu and Sun Wanjun, Characteristics and source of heavy oils in southwestern slope of Songliao Basin. Petroleum exploration and development, 2002,29(2):45~48]
    [25] 窦立荣, 徐树宝, 祝玉衡, 平学聪. 二连盆地重质稠油藏成因及地化特征. 石油学报, 1995, 2: 1~7[Dou Lirong, Xu Shubao, Zhu Yuheng,et al. Geochemical characteristics of heavy oils and reservoir formation in Erlian Basin. Petrolei,1995,16(2):1~7]
    [26] Moldowan J M and McCaffrey M A. A novel microbial hydrocarbon degradation pathway revealed by hopane demethylation in a petroleum reservoir. Geochimica et Cosmochimica Acta, 1995, 59(9):1891~1894
    [27] 包建平.未降解原油和生油岩中的25-降藿烷系列. 科学通报, 1996, 41(20):1875~1878[Bao Jianping. 25-norhopanes in unbiodegraded oils and source rocks. Chinese bulletin of sciences, 1996,41(20):1875~1878]
    [28] 包建平,梅博文.25-降藿烷系列的"异常"分布及其成因. 沉积学报, 1997, 15(2):179~183[Bao Jianping and Mei Bowen. Unconventional distribution and formation of 25-norhopanes. Acta sedimentologica Sinica,1997,15(2):179~183]
    [29] Tissot B P and Welte D H. Petroleum Formation and Occurrence. Berlin: Springer-Verlag, 1978
    [30] Peters K E, Moldowan J M. The Biomarkers Guide: interpreting molecular fossils in petroleum and ancient sediments. New York: Prentice Hall, 1993
    [31] Volkman J K, Alexander R, Kagi R I, et al. A geochemical reconstruction of oil generation in the Barrow Sub-basin of Western Australia. Geochimic et Cosmochimica Acta, 1983a, 47: 2091~2105
    [32] Volkman J K, Alexander R, Kagi R I, et al. Demethylated hopanes in crude oils and their applications in petroleum geochemistry. Geochimica et Cosmochimica Acta, 1983b, 47: 785~794
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  • 收稿日期:  2003-10-14
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目录

    济阳拗陷特殊生物降解油的初步研究

      基金项目:  中国科学院创新知识工程项目(KZCX1-SW-18);国家基础研究“973”项目(G1999043308)资助.
      作者简介:

      卢鸿 男 1971年出生 副研究员 石油地球化学和有机地球化学

    • 中图分类号: P593

    摘要: 济阳拗陷草古100平19井奥陶系储层原油,饱和烃馏分均已损失殆尽,仅残余藿烷系列化合物;同时,芳烃馏分化合物也已损失殆尽,仅残余三芳甾烷系列化合物。上述芳烃化合物俱已损失殆尽的蚀变特征,在相关文献中的报道较为少见。原油中不受水洗作用影响的正构烷烃和不受生物降解作用影响的有机硫化合物(苯并噻吩和二苯并噻吩)均已损失殆尽,显然暗示了原油蚀变是遭受水洗作用和生物降解作用共同作用的结果。原油芳烃馏分的“UCM”鼓包幅度明显大于饱和烃馏分的“UCM”鼓包,暗示了芳烃化合物的降解速率平行甚至超过饱和烃的降解速率。原油中低分子量芳烃化合物的快速降解,暗示了油藏可能是在氧化条件下而非在还原条件下发生蚀变的。

    English Abstract

    卢鸿, 彭平安, 徐兴友, 张林晔. 济阳拗陷特殊生物降解油的初步研究[J]. 沉积学报, 2004, 22(4): 694-699.
    引用本文: 卢鸿, 彭平安, 徐兴友, 张林晔. 济阳拗陷特殊生物降解油的初步研究[J]. 沉积学报, 2004, 22(4): 694-699.
    LU Hong, PENG Ping an, XU Xing you, ZHANG Lin ye. Preliminary Study on the Severely Biodegraded Crude Oil in Jiyang Depression, China[J]. Acta Sedimentologica Sinica, 2004, 22(4): 694-699.
    Citation: LU Hong, PENG Ping an, XU Xing you, ZHANG Lin ye. Preliminary Study on the Severely Biodegraded Crude Oil in Jiyang Depression, China[J]. Acta Sedimentologica Sinica, 2004, 22(4): 694-699.
    参考文献 (32)

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